The 33-year-old star and her 6-year-old daughter were accompanied by her mother Kathy, who has been spotted with them numerous times since her split from Tom Cruise.
PLAY IT NOW: How Did Katie Holmes Tell Tom Cruise She Wanted A Divorce?
Suri appeared excited to visit the zoo's residents, especially when she got to feed the alpacas and the goats. She was seen sharing the animal food with other children at the zoo.
Later on Wednesday night, Katie turned up her new single lady style hitting the town in tight black leather pants, heels and a matching white blouse and jacket.
VIEW THE PHOTOS: Katie Holmes Steps Out After Leaving Tom Cruise
According to Us Weekly, the actress - who was seen flanked by bodyguards while walking the NYC streets - had dinner with a friend.
Check out Katie's stylish evening look HERE!
And for more on how Katie pulled off her own 'Mission: Impossible,' blindsiding Tom Cruise with her divorce filing - which included staff firings and secret cell phones - CLICK HERE!
VIEW THE PHOTOS: Stars Who Split In 2012
-- Jesse Spero
Copyright 2012 by NBC Universal, Inc. All rights reserved.
This material may not be published, broadcast, rewritten or redistributed.
VIEW THE PHOTOS: Tom Cruise & Katie Holmes: A Look Back
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